Brahim Guizal and Mauro Antezza
We show that the electromagnetic forces generated by the excitations of a mode in graphene-based optomechanical systems are highly tunable by varying the graphene chemical potential, and orders of magnitude stronger than usual non-graphene-based devices, in both attractive and repulsive regimes. We analyze coupled waveguides made of two parallel graphene sheets, either suspended or supported by dielectric slabs, and study the interplay between the light-induced force and the Casimir-Lifshitz interaction. These findings pave the way to advanced possibilities of control and fast modulation for optomechanical devices and sensors at the nano- and microscales.
DOI
Friday, April 29, 2016
Direct observation of intermediate states in model membrane fusion
Andrea Keidel, Tobias F. Bartsch & Ernst-Ludwig Florin
We introduce a novel assay for membrane fusion of solid supported membranes on silica beads and on coverslips. Fusion of the lipid bilayers is induced by bringing an optically trapped bead in contact with the coverslip surface while observing the bead’s thermal motion with microsecond temporal and nanometer spatial resolution using a three-dimensional position detector. The probability of fusion is controlled by the membrane tension on the particle. We show that the progression of fusion can be monitored by changes in the three-dimensional position histograms of the bead and in its rate of diffusion. We were able to observe all fusion intermediates including transient fusion, formation of a stalk, hemifusion and the completion of a fusion pore. Fusion intermediates are characterized by axial but not lateral confinement of the motion of the bead and independently by the change of its rate of diffusion due to the additional drag from the stalk-like connection between the two membranes. The detailed information provided by this assay makes it ideally suited for studies of early events in pure lipid bilayer fusion or fusion assisted by fusogenic molecules.
DOI
We introduce a novel assay for membrane fusion of solid supported membranes on silica beads and on coverslips. Fusion of the lipid bilayers is induced by bringing an optically trapped bead in contact with the coverslip surface while observing the bead’s thermal motion with microsecond temporal and nanometer spatial resolution using a three-dimensional position detector. The probability of fusion is controlled by the membrane tension on the particle. We show that the progression of fusion can be monitored by changes in the three-dimensional position histograms of the bead and in its rate of diffusion. We were able to observe all fusion intermediates including transient fusion, formation of a stalk, hemifusion and the completion of a fusion pore. Fusion intermediates are characterized by axial but not lateral confinement of the motion of the bead and independently by the change of its rate of diffusion due to the additional drag from the stalk-like connection between the two membranes. The detailed information provided by this assay makes it ideally suited for studies of early events in pure lipid bilayer fusion or fusion assisted by fusogenic molecules.
DOI
Mechanical Resonators for Quantum Optomechanics Experiments at Room Temperature
R. A. Norte, J. P. Moura, and S. Gröblacher
All quantum optomechanics experiments to date operate at cryogenic temperatures, imposing severe technical challenges and fundamental constraints. Here, we present a novel design of on-chip mechanical resonators which exhibit fundamental modes with frequencies f and mechanical quality factors Qm sufficient to enter the optomechanical quantum regime at room temperature. We overcome previous limitations by designing ultrathin, high-stress silicon nitride (Si3N4) membranes, with tensile stress in the resonators’ clamps close to the ultimate yield strength of the material. By patterning a photonic crystal on the SiN membranes, we observe reflectivities greater than 99%. These on-chip resonators have remarkably low mechanical dissipation, with Qm∼108, while at the same time exhibiting large reflectivities. This makes them a unique platform for experiments towards the observation of massive quantum behavior at room temperature.
DOI
All quantum optomechanics experiments to date operate at cryogenic temperatures, imposing severe technical challenges and fundamental constraints. Here, we present a novel design of on-chip mechanical resonators which exhibit fundamental modes with frequencies f and mechanical quality factors Qm sufficient to enter the optomechanical quantum regime at room temperature. We overcome previous limitations by designing ultrathin, high-stress silicon nitride (Si3N4) membranes, with tensile stress in the resonators’ clamps close to the ultimate yield strength of the material. By patterning a photonic crystal on the SiN membranes, we observe reflectivities greater than 99%. These on-chip resonators have remarkably low mechanical dissipation, with Qm∼108, while at the same time exhibiting large reflectivities. This makes them a unique platform for experiments towards the observation of massive quantum behavior at room temperature.
DOI
Ultralow-Noise SiN Trampoline Resonators for Sensing and Optomechanics
Christoph Reinhardt, Tina Müller, Alexandre Bourassa, and Jack C. Sankey
In force sensing, optomechanics, and quantum motion experiments, it is typically advantageous to create lightweight, compliant mechanical elements with the lowest possible force noise. Here, we report the fabrication and characterization of high-aspect-ratio, nanogram-scale Si3N4 “trampolines” having quality factors above 4×107 and ringdown times exceeding 5 min (mHz linewidth). These devices exhibit thermally limited force noise sensitivities below 20 aN/Hz1/2 at room temperature, which is the lowest among solid-state mechanical sensors. We also characterize the suitability of these devices for high-finesse cavity readout and optomechanics applications, finding no evidence of surface or bulk optical losses from the processed nitride in a cavity achieving finesse 40,000. These parameters provide access to a single-photon cooperativity C0∼8 in the resolved-sideband limit, wherein a variety of outstanding optomechanics goals become feasible.
DOI
In force sensing, optomechanics, and quantum motion experiments, it is typically advantageous to create lightweight, compliant mechanical elements with the lowest possible force noise. Here, we report the fabrication and characterization of high-aspect-ratio, nanogram-scale Si3N4 “trampolines” having quality factors above 4×107 and ringdown times exceeding 5 min (mHz linewidth). These devices exhibit thermally limited force noise sensitivities below 20 aN/Hz1/2 at room temperature, which is the lowest among solid-state mechanical sensors. We also characterize the suitability of these devices for high-finesse cavity readout and optomechanics applications, finding no evidence of surface or bulk optical losses from the processed nitride in a cavity achieving finesse 40,000. These parameters provide access to a single-photon cooperativity C0∼8 in the resolved-sideband limit, wherein a variety of outstanding optomechanics goals become feasible.
DOI
Raman activated cell sorting
Yizhi Song, Huabing Yin, Wei E Huang
Single cell Raman spectra (SCRS) are intrinsic biochemical profiles and ‘chemical images’ of single cells which can be used to characterise phenotypic changes, physiological states and functions of cells. On the base of SCRS, Raman activated cell sorting (RACS) provides a label-free cell sorting approach, which can link single cells to their chemical or phenotypic profiles. Overcoming naturally weak Raman signals, establishing Raman biomarker as sorting criteria to RACS and improving specific sorting technology are three challenges of developing RACS. Advances on Raman spectroscopy such as stimulated Raman scattering (SRS) and pre-screening helped to increase RACS sorting speed. Entire SCRS can be characterised using pattern recognition methods, and specific Raman bands can be extracted as biomarkers for RACS. Recent advances on cell sorting technologies based on microfluidic device and surface-ejection enable accurate and reliable single cell sorting from complex samples. A high throughput RACS will be achievable in near future by integrating fast Raman detection system such as SRS with microfluidic RACS and Raman activated cell ejection (RACE).
DOI
Single cell Raman spectra (SCRS) are intrinsic biochemical profiles and ‘chemical images’ of single cells which can be used to characterise phenotypic changes, physiological states and functions of cells. On the base of SCRS, Raman activated cell sorting (RACS) provides a label-free cell sorting approach, which can link single cells to their chemical or phenotypic profiles. Overcoming naturally weak Raman signals, establishing Raman biomarker as sorting criteria to RACS and improving specific sorting technology are three challenges of developing RACS. Advances on Raman spectroscopy such as stimulated Raman scattering (SRS) and pre-screening helped to increase RACS sorting speed. Entire SCRS can be characterised using pattern recognition methods, and specific Raman bands can be extracted as biomarkers for RACS. Recent advances on cell sorting technologies based on microfluidic device and surface-ejection enable accurate and reliable single cell sorting from complex samples. A high throughput RACS will be achievable in near future by integrating fast Raman detection system such as SRS with microfluidic RACS and Raman activated cell ejection (RACE).
DOI
Tuesday, April 26, 2016
Universal spin-momentum locked optical forces
Farid Kalhor, Thomas Thundat and Zubin Jacob
Evanescent electromagnetic waves possess spin-momentum locking, where the direction of propagation (momentum) is locked to the inherent polarization of the wave (transverse spin). We study the optical forces arising from this universal phenomenon and show that the fundamental origin of recently reported non-trivial optical chiral forces is spin-momentum locking. For evanescent waves, we show that the direction of energy flow, the direction of decay, and the direction of spin follow a right hand rule for three different cases of total internal reflection, surface plasmon polaritons, and HE11 mode of an optical fiber. Furthermore, we explain how the recently reported phenomena of lateral optical force on chiral and achiral particles are caused by the transverse spin of the evanescent field and the spin-momentum locking phenomenon. Finally, we propose an experiment to identify the unique lateral forces arising from the transverse spin in the optical fiber and point to fundamental differences of the spin density from the well-known orbital angular momentum of light. Our work presents a unified view on spin-momentum locking and how it affects optical forces on chiral and achiral particles.
DOI
Evanescent electromagnetic waves possess spin-momentum locking, where the direction of propagation (momentum) is locked to the inherent polarization of the wave (transverse spin). We study the optical forces arising from this universal phenomenon and show that the fundamental origin of recently reported non-trivial optical chiral forces is spin-momentum locking. For evanescent waves, we show that the direction of energy flow, the direction of decay, and the direction of spin follow a right hand rule for three different cases of total internal reflection, surface plasmon polaritons, and HE11 mode of an optical fiber. Furthermore, we explain how the recently reported phenomena of lateral optical force on chiral and achiral particles are caused by the transverse spin of the evanescent field and the spin-momentum locking phenomenon. Finally, we propose an experiment to identify the unique lateral forces arising from the transverse spin in the optical fiber and point to fundamental differences of the spin density from the well-known orbital angular momentum of light. Our work presents a unified view on spin-momentum locking and how it affects optical forces on chiral and achiral particles.
DOI
Graphene-based plasmonic force switch
M. Ghorbanzadeh, S. Darbari and M. K. Moravvej-Farshi
We take advantage of a Kretschmann configuration to design a plasmonic force switch. It consists of a prism/Au/SiO2 stack topped by a gated graphene sheet, as an electrically active optofluidic particle sorting system. We show that using a small gate voltage, one can switch the plasmon-wave induced force on a target particle, and hence its velocity. Simulations show that by electrical tuning of the grapheneelectrochemical potential in a narrow range of ∼65 meV—i.e., equivalent to an applied gate voltage of ∼4.3 V—the graphenesurface plasmons can absorb the Ausurface plasmons, switching off the plasmonic force exerted on the target particle with an ON/OFF ratio of more than 20. Numerical results also show that the maximum sensitivity of the particle's velocity to the graphene electrochemical potential is ∼1136 μm/eV-s. The proposed electrically active plasmonic force switch offers opportunities in developing tunable on-chip optical micromanipulations with multiple parallel functionalities and low power consumption.
DOI
We take advantage of a Kretschmann configuration to design a plasmonic force switch. It consists of a prism/Au/SiO2 stack topped by a gated graphene sheet, as an electrically active optofluidic particle sorting system. We show that using a small gate voltage, one can switch the plasmon-wave induced force on a target particle, and hence its velocity. Simulations show that by electrical tuning of the grapheneelectrochemical potential in a narrow range of ∼65 meV—i.e., equivalent to an applied gate voltage of ∼4.3 V—the graphenesurface plasmons can absorb the Ausurface plasmons, switching off the plasmonic force exerted on the target particle with an ON/OFF ratio of more than 20. Numerical results also show that the maximum sensitivity of the particle's velocity to the graphene electrochemical potential is ∼1136 μm/eV-s. The proposed electrically active plasmonic force switch offers opportunities in developing tunable on-chip optical micromanipulations with multiple parallel functionalities and low power consumption.
DOI
Motion of Optically Heated Spheres at the Water–Air Interface
A. Girot, N. Danné, A. Würger, T. Bickel, F. Ren, J. C. Loudet, and B. Pouligny
A micrometer-sized spherical particle classically equilibrates at the water–air interface in partial wetting configuration, causing about no deformation to the interface. In condition of thermal equilibrium, the particle just undergoes faint Brownian motion, well visible under a microscope. We report experimental observations when the particle is made of a light-absorbing material and is heated up by a vertical laser beam. We show that, at small laser power, the particle is trapped in on-axis configuration, similarly to 2-dimensional trapping of a transparent sphere by optical forces. Conversely, on-axis trapping becomes unstable at higher power. The particle escapes off the laser axis and starts orbiting around the axis. We show that the laser-heated particle behaves as a microswimmer with velocities on the order of several 100 μm/s with just a few milliwatts of laser power.
DOI
A micrometer-sized spherical particle classically equilibrates at the water–air interface in partial wetting configuration, causing about no deformation to the interface. In condition of thermal equilibrium, the particle just undergoes faint Brownian motion, well visible under a microscope. We report experimental observations when the particle is made of a light-absorbing material and is heated up by a vertical laser beam. We show that, at small laser power, the particle is trapped in on-axis configuration, similarly to 2-dimensional trapping of a transparent sphere by optical forces. Conversely, on-axis trapping becomes unstable at higher power. The particle escapes off the laser axis and starts orbiting around the axis. We show that the laser-heated particle behaves as a microswimmer with velocities on the order of several 100 μm/s with just a few milliwatts of laser power.
DOI
Monday, April 25, 2016
Ignition and combustion characteristics of jet fuel liquid film containing graphene powders at meso-scale
Xuefeng Huang, Shengji Li
At meso-scale, ignition and combustion characteristics of jet fuel liquid film containing graphene powders were investigated. Jet fuel/graphene suspensions were prepared, and sprayed to produce the liquid film. Liquid film was ignited by optical tweezers, five distinctive stages including graphene trap, ignition and combustion of graphene, bubble formation, jet fuel vaporization and bubble growth, bubble rupture and combustion of liquid film were identified. Ignition of graphene is prior to jet fuel. The combustion heat of graphene serves a heat source to accelerate the vaporization of jet fuel. The graphene serves as a nucleation point to form a bubble. Expansion of both combustion products and jet fuel vapor result in the bubble growth. The thickness of bubble boundary layer depends on graphene concentration. As the bubble escaped, liquid film ruptured and micro-explosion occurred. Jet fuel was then ignited, and combusted sustainably till burnt out. During combustion, the flame front fluctuated slightly, indicating good flame stability. Finally, a schematic physical model was presented to analyze the inductive mechanism of graphene for ignition and combustion of jet fuel liquid film by optical tweezers.
DOI
At meso-scale, ignition and combustion characteristics of jet fuel liquid film containing graphene powders were investigated. Jet fuel/graphene suspensions were prepared, and sprayed to produce the liquid film. Liquid film was ignited by optical tweezers, five distinctive stages including graphene trap, ignition and combustion of graphene, bubble formation, jet fuel vaporization and bubble growth, bubble rupture and combustion of liquid film were identified. Ignition of graphene is prior to jet fuel. The combustion heat of graphene serves a heat source to accelerate the vaporization of jet fuel. The graphene serves as a nucleation point to form a bubble. Expansion of both combustion products and jet fuel vapor result in the bubble growth. The thickness of bubble boundary layer depends on graphene concentration. As the bubble escaped, liquid film ruptured and micro-explosion occurred. Jet fuel was then ignited, and combusted sustainably till burnt out. During combustion, the flame front fluctuated slightly, indicating good flame stability. Finally, a schematic physical model was presented to analyze the inductive mechanism of graphene for ignition and combustion of jet fuel liquid film by optical tweezers.
DOI
Optical Trapping-Formed Colloidal Assembly with Horns Extended to the Outside of a Focus through Light Propagation
Tetsuhiro Kudo, Shun-Fa Wang, Ken-ichi Yuyama, and Hiroshi Masuhara
We report optical trapping and assembling of colloidal particles at a glass/solution interface with a tightly focused laser beam of high intensity. It is generally believed that the particles are gathered only in an irradiated area where optical force is exerted on the particles by laser beam. Here we demonstrate that, the propagation of trapping laser from the focus to the outside of the formed assembly leads to expansion of the assembly much larger than the irradiated area with sticking out rows of linearly aligned particles like horns. The shape of the assembly, its structure, and the number of horns can be controlled by laser polarization. Optical trapping study utilizing the light propagation will open a new avenue for assembling and crystallizing quantum dots, metal nanoparticles, molecular clusters, proteins, and DNA.
DOI
We report optical trapping and assembling of colloidal particles at a glass/solution interface with a tightly focused laser beam of high intensity. It is generally believed that the particles are gathered only in an irradiated area where optical force is exerted on the particles by laser beam. Here we demonstrate that, the propagation of trapping laser from the focus to the outside of the formed assembly leads to expansion of the assembly much larger than the irradiated area with sticking out rows of linearly aligned particles like horns. The shape of the assembly, its structure, and the number of horns can be controlled by laser polarization. Optical trapping study utilizing the light propagation will open a new avenue for assembling and crystallizing quantum dots, metal nanoparticles, molecular clusters, proteins, and DNA.
DOI
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